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Humanization STEM™ Developability pH-dependent release

We rebuilt one of the world’s best-selling antibodies — and published what went wrong on the way

Infliximab is clinically validated, commercially enormous, and biophysically awkward: a mouse–human chimera with documented Fab–Fab self-association. We humanized it, matured it with STEM™, and found that maturation alone did not fix its self-association. This is what we did next, with every number.

2.8×more potent than chimeric infliximab
4.8×more potent than adalimumab
19.33 → −1.67AC-SINS Δλmax (nm)
>1800×faster off-rate at pH 5.8

All data from our preprint: doi:10.64898/2026.08.18.745573 (bioRxiv, 19 August 2026). Preprint — not certified by peer review.

Why we picked a molecule we could not flatter

Most CRO case studies use a target the CRO chose because it was winnable. We wanted the opposite: a molecule whose weaknesses are already in the literature, whose benchmark is a marketed drug, and where anyone can check our claim against a competitor they already know.

Infliximab qualifies on all three counts. It is a mouse–human chimeric anti-TNFα IgG1 with murine variable domains, a known driver of human anti-chimeric antibody responses. It undergoes reversible self-association through Fab–Fab interactions, which is documented in structural and solution studies and is exactly the property that makes a molecule hard to formulate at high concentration. And it requires prolonged intravenous infusion.

In other words: a clinically proven binding site attached to a body that a modern developability panel would flag. That is the situation many of our clients are actually in.

What we did, in three moves

1. Humanization

The infliximab CDRs were grafted onto human germline acceptor frameworks. We selected IGKV6-21 and IGHV3-72 by IgBLAST on the basis of sequence identity and preservation of canonical loop structure. The resulting humanized antibody, hInfliximab, retained TNFα binding but lost potency — IC50 166.1 ng/mL against 96.8 ng/mL for the chimeric parent.

That drop is normal and it is the reason humanization and maturation are usually scoped together rather than sequentially.

2. STEM™ affinity maturation

We applied STage-Enhanced Maturation to hInfliximab. Focused libraries were designed at preselected CDR positions using the amino acid usage and positional frequencies observed in human antibodies, biasing the sequence toward a human-like profile rather than away from one. Library complexity was held within the electroporation capacity of roughly 1 × 1010 cfu.

Every selection round was heat-challenged and subtracted against a panel of polyspecificity reagents — baculovirus particles, dsDNA, ovalbumin, HSP90-Fc and KLH — before panning on TNFα. The matured clone hInBG4 recovered and exceeded parental potency at IC50 42.0 ng/mL.

3. Targeted CDR substitution — the step we would rather not have needed

Developability profiling then told us something we did not want to hear. hInBG4 had inherited the parental self-association: an AC-SINS Δλmax of 9.00 nm, against 19.33 nm for infliximab itself. The affinity work had succeeded; the biophysics had not.

So we treated hInBG4 as a new scaffold, built a panel of targeted single and combined CDR substitutions, and profiled every variant on four orthogonal readouts — AC-SINS, BVP ELISA, SE-HPLC and transient expression. Three cleared all four.

The result

Potency versus self-association for infliximab-derived variants Scatter plot of TNF-alpha neutralization IC50 against AC-SINS self-association. Engineered clones LW2Y, LW2YR2S and LW2YHR1K sit in the desirable low-IC50, low-self-association corner, while chimeric infliximab and the STEM-matured intermediate hInBG4 sit high on the self-association axis. desirable −50 510 1520 050 100150 TNFα neutralization IC₅₀ (ng/mL) — lower is more potent → AC-SINS Δλmax (nm) — lower is less self-associating targeted CDR substitution Infliximab chimeric parent hInfliximab Adalimumab hInBG4 STEM™ output LW2Y LW2YR2S LW2YHR1K reference STEM™ matured final engineered
STEM™ maturation moved the molecule left (more potent) but not down — hInBG4 kept the parental self-association liability. Targeted CDR substitution moved it down without giving the potency back. Data from Table 1 of the preprint.
CloneTNFα neutralization
IC50 (ng/mL)
Self-association
AC-SINS Δλmax (nm)
Non-specificity
BVP ELISA ratio
LW2Y34.5−1.671.5
LW2YHR1K33.20.331.3
LW2YR2S45.4−0.331.5
hInBG4 — STEM™ output42.09.002.3
hInfliximab — humanized parent166.1−4.001.1
Infliximab — chimeric parent96.819.331.3
Adalimumab — benchmark167.0−1.331.6

LW2Y neutralizes TNFα 2.8× more potently than chimeric infliximab and 4.8× more potently than adalimumab, while self-associating less than either.

SE-HPLC showed sharp, symmetrical monomer peaks for the engineered variants where infliximab and hInBG4 both tailed, with NISTmAb RM 8671 run as a reference standard. Transient expression in HEK293 rose from roughly 50 µg/mL for the humanized parent to the high 70s and 80s for the engineered clones.

What each assay is actually predicting

AssayWhat a bad number would cost you later
AC-SINSWeak self-interaction correlates with aggregation, high viscosity at concentration, and poor colloidal stability — the difference between a subcutaneous product and an infusion.
BVP ELISAPolyspecificity against a heterogeneous membrane surface; high ratios track with fast clearance and poor PK.
SE-HPLCHigh-molecular-weight species and peak tailing — the aggregate burden a regulator will ask about.
Transient expressionA first, cheap read on whether the molecule will express at manufacturing scale.

pH-dependent antigen release, engineered rather than traded for

An antibody that holds antigen tightly in plasma but lets go in the acidified endosome can be recycled by FcRn and bind again. Where a programme is limited by target-mediated drug disposition, that behaviour can reduce antigen accumulation and, in some cases, dose and dosing frequency.

The published attempts at pH-dependent anti-TNFα antibodies have generally used histidine scanning, and in some cases the pH switch came at the cost of neutral-pH binding. The point of the readout below is that LW2Y did not pay that price.

TNF-alpha dissociation rate at pH 7.4 versus pH 5.8 Log-scale dot plot of dissociation rate constants measured by biolayer interferometry. LW2Y dissociates more than 1800-fold faster at pH 5.8 than at pH 7.4; chimeric infliximab shows no pH-dependent release. 10⁻⁷10⁻⁶10⁻⁵10⁻⁴10⁻³ Dissociation rate k dis (s⁻¹) — log scale fold acceleration LW2YLW2YR2SLW2YHR1K AdalimumabhInfliximabInfliximab below detection limit >180018.31.9 2161.80.69 no release dissociation at pH 7.4 (plasma) dissociation at pH 5.8 (endosome)
Longer bars mean a bigger pH switch. LW2Y holds antigen almost irreversibly at pH 7.4 and lets go at pH 5.8; chimeric infliximab moves the wrong way. Measured in-house by Octet BLI, association at pH 7.4 in every case. Data from Table 2 of the preprint.
CloneKD (nM) pH 7.4ka (M−1s−1)kdis (s−1) pH 7.4kdis (s−1) pH 5.8Fold
LW2Y<0.0011.06 × 105<1.0 × 10−71.80 × 10−4>1800
LW2YR2S0.0561.74 × 1059.82 × 10−61.80 × 10−418.3
LW2YHR1K0.5391.76 × 1059.49 × 10−51.77 × 10−41.9
Adalimumab0.0121.72 × 1052.01 × 10−64.35 × 10−4216
hInfliximab0.7522.12 × 1051.60 × 10−42.82 × 10−41.8
Infliximab1.0092.17 × 1052.19 × 10−41.51 × 10−40.69

Measured in-house by biolayer interferometry on the Octet platform. TNFα was captured on streptavidin biosensors, association was performed at pH 7.4 in every case, and only the dissociation buffer was changed. LW2Y’s off-rate at pH 7.4 fell below the assay’s reliable detection limit, so its fold-change is reported as a lower bound.

Immunogenicity: what we can and cannot claim

We analysed the VH and VL sequences of infliximab, hInfliximab and every engineered variant with the IEDB Deimmunization tool in peptide mutant prediction mode, at a median percentile rank threshold of 20.

One peptide in the light chain of chimeric infliximab (DILLTQSPAILSVSP, median percentile rank 16.5) met the threshold as a predicted MHC class II–restricted epitope. No peptide met the threshold in the light chains of hInfliximab, hInBG4, LW2Y, LW2YR2S or LW2YHR1K, nor in any heavy-chain sequence.

Within the limits of an in silico method: humanization removed one predicted T-cell epitope and the CDR-level engineering introduced no new high-risk ones. That is a sequence-liability result, not a clinical immunogenicity result, and we will not present it as one.

What this demonstrates — and what it does not

This programme was run to test our own platform end to end on a molecule that would not flatter it. It shows three things we can do on your antibody:

  • Humanize onto human germline frameworks without stranding the paratope — and recover the potency the graft costs.
  • Mature affinity while screening developability inside the campaign, not after it, so polyreactive and thermally fragile clones never reach the shortlist.
  • Engineer a specific biophysical property on demand — here pH-dependent release — and verify it kinetically rather than infer it.

It also shows the honest shape of the work. STEM™ did not fix everything in one pass. Self-association survived maturation and had to be engineered out deliberately in a second round guided by measurement. Any platform that claims otherwise on every molecule is describing a marketing process, not a laboratory one.

LW2Y is presented here as evidence of capability. It is a demonstration lead from an internal programme, not a product offered for licensing on this page.

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